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掺镱飞秒激光晶体研究进展

孙士家 娄斐 林州斌 钟德高 滕冰

孙士家, 娄斐, 林州斌, 等. 掺镱飞秒激光晶体研究进展[J]. 强激光与粒子束, 2020, 32: 011009. doi: 10.11884/HPLPB202032.190451
引用本文: 孙士家, 娄斐, 林州斌, 等. 掺镱飞秒激光晶体研究进展[J]. 强激光与粒子束, 2020, 32: 011009. doi: 10.11884/HPLPB202032.190451
Sun Shijia, Lou Fei, Lin Zhoubin, et al. Progress of the research on Yb3+-doped femtosecond laser crystals[J]. High Power Laser and Particle Beams, 2020, 32: 011009. doi: 10.11884/HPLPB202032.190451
Citation: Sun Shijia, Lou Fei, Lin Zhoubin, et al. Progress of the research on Yb3+-doped femtosecond laser crystals[J]. High Power Laser and Particle Beams, 2020, 32: 011009. doi: 10.11884/HPLPB202032.190451

掺镱飞秒激光晶体研究进展

doi: 10.11884/HPLPB202032.190451
基金项目: 国家自然科学基金项目(61705231,51972181);山东省自然科学基金重大基础研究项目(ZR2018ZB0650)
详细信息
    作者简介:

    孙士家(1987—),男,硕士,工程师,从事新型激光晶体研究;ssj1027@126.com

    通讯作者:

    滕 冰(1968—),女,博士,教授,从事新型光电功能晶体材料研究;5108tb@163.com

  • 中图分类号: O799

Progress of the research on Yb3+-doped femtosecond laser crystals

  • 摘要: 飞秒激光在军事、医学、通讯、加工等领域有着重要应用,已经成为新世纪激光技术领域的研究热点。得益于激光二极管(LD)的快速发展,以LD作为泵浦源成为新型全固态飞秒激光器的发展趋势。Yb3+离子掺杂的激光晶体材料因其独特的能级结构、宽带吸收与发射等优势,逐渐成为LD直接泵浦并实现1.0 μm飞秒激光输出的重要增益介质。详细总结了当前掺Yb3+飞秒激光晶体的研究进展,分析了目前存在的主要问题,给出了未来飞秒激光晶体发展的两个建议方向:高效率小功率飞秒激光和大功率高能量飞秒激光。以Yb3+:Sr3Y2(BO3)4晶体为例,详细研究了其晶体生长、光谱、连续与飞秒激光性能,并实现了中心波长在1 060 nm处脉宽为116 fs,平均输出功率为1.08 W,光光转换效率为33.1%的高效率飞秒激光输出,表明Yb3+:Sr3Y2(BO3)4及其同体系晶体是一类优异的高效率飞秒激光材料。
  • 图  1  采用提拉法生长的原子数分数为3%的Yb:SYB晶体[89]

    Figure  1.  3at.%Yb:SYB crystals grown by Czochralski method[89]

    图  2  原子数分数为3%的Yb:SYB晶体的偏振吸收截面[89]

    Figure  2.  Polarized absorption cross-sections of 3at.%Yb:SYB crystal[89]

    图  3  原子数分数为3%的Yb:SYB晶体的偏振发射截面[89]

    Figure  3.  Polarized emission cross-sections of 3at.%Yb:SYB crystal[89]

    图  4  原子数分数为3%的Yb:SYB晶体的荧光衰减曲线[89]

    Figure  4.  Fluorescence decay curve of 3at.%Yb:SYB crystal[89]

    图  5  激光实验装置示意图[89]

    Figure  5.  Schematic diagram of laser experimental setup[89]

    图  6  原子数分数为3%的Yb:SYB晶体连续激光泵浦与输出功率[89]

    Figure  6.  CW laser output versus incident pump powers of 3at.%Yb:SYB crystal[89]

    图  7  原子数分数为3%的Yb:SYB晶体激光发射谱图[89]

    Figure  7.  Laser emission spectra of 3at.%Yb:SYB crystal[89]

    图  8  克尔透镜锁模激光实验装置示意图[90]

    Figure  8.  Experimental setup of Kerr-lens mode-locked laser[90]

    图  9  原子数分数为3%的Yb:SYB晶体平均输出功率与脉冲宽度[90]

    Figure  9.  Average output power and pulse duration of 3at.%Yb:SYB laser[90]

    图  10  原子数分数为3%的Yb:SYB晶体脉冲激光自相关曲线与光谱图[90]

    Figure  10.  Autocorrelation trace and spectrum of 3at.%Yb:SYB pulse laser[90]

    图  11  采用提拉法生长的原子数分数为11%的Yb:SYB晶体[91]

    Figure  11.  11at.%Yb:SYB crystal grown by Czochralski method[91]

    图  12  SESAM锁模激光实验装置示意图[91]

    Figure  12.  Experimental setup of the SESAM mode-locked laser[91]

    图  13  原子数分数为11%的Yb:SYB晶体锁模激光平均输出功率与泵浦功率[91]

    Figure  13.  Average output versus incident pump powers of 11at.%Yb:SYB crystal[91]

    图  14  原子数分数为11%的Yb:SYB晶体锁模激光光谱与自相关曲线[91]

    Figure  14.  Autocorrelation traces and laser emission spectra of 11at.%Yb:SYB mode-locked pulses[91]

    图  15  采用提拉法生长的原子数分数为6.3%的Yb:SGB晶体[94]

    Figure  15.  6.3at.%Yb:SGB crystal grown by Czochralski method[94]

    图  16  原子数分数为6.3%的Yb:SGB晶体的结构特征[94]

    Figure  16.  The structure of 6.3at.%Yb:SGB crystal[94]

    图  17  室温下原子数分数为6.3%的Yb:SGB晶体的偏振吸收截面和荧光光谱[94]

    Figure  17.  Polarized absorption cross-sections and fluorescence spectra of 6.3at.%Yb:SGB at 300 K[94]

    图  18  原子数分数为6.3%的Yb:SGB晶体77 K温度下荧光光谱以及Yb3+离子能级图[94]

    Figure  18.  Fluorescence spectra of 6.3at.%Yb:SGB crystal at 77 K and energy level schema of Yb3+ ions[94]

    图  19  原子数分数为6.3%的Yb:SGB晶体的荧光衰减曲线[94]

    Figure  19.  Fluorescence decay curve of 6.3at.%Yb:SGB crystal[94]

    图  20  原子数分数为6.3%的Yb:SGB晶体的偏振发射截面与增益截面[94]

    Figure  20.  Polarized emission and gain cross-sections of 6.3at.%Yb:SGB crystal[94]

    图  21  原子数分数为6.3%的Yb:SGB晶体的连续激光输出功率与吸收泵浦功率[94]

    Figure  21.  CW output versus absorbed pump powers of 6.3at.%Yb:SGB crystal[94]

    图  22  原子数分数为6.3%的Yb:SGB晶体连续激光发射谱[94]

    Figure  22.  Laser emission spectra of 6.3at.%Yb:SGB crystal[94]

    表  1  掺Yb3+飞秒激光晶体的光谱与激光参数

    Table  1.   Spectra and laser parameters of Yb3+-doped femtosecond laser crystals

    matrix crystalabsorption spectrum FWHM/nmemission spectrum FWHM/nmwavelength/nmpulse width/fsaverage power/mWoptical-optical conversion efficiency/%reference
    YCa4O(BO3)3 3 44 1 055
    1 050
    35
    46
    36
    46
    2.6
    4.2
    [14-15]
    GdCa4O(BO3)3 3 44 1 045
    1 030
    90
    350
    40
    2
    [16-17]
    Sr3Y(BO3)3 6 60 1 062
    1 068
    69
    86
    80
    300
    7.3
    12
    [18-19]
    YAl3(BO3)4 22 25 1 050 87 61 2.5 [20-21]
    LaSc3(BO3)4 25 33 1 053 67
    58
    39
    73
    2
    3.7
    [22-23]
    KY(WO4)2 3.5 24 1 039
    1 033
    65
    114
    22
    5 000
    2
    33.3
    [24-25]
    KGd(WO4)2 3.5 25 1 040
    1 038
    67
    162
    3 000
    8 800
    10
    32.1
    [26-27]
    CaGdAlO4 6 60 1 063
    1 050
    32
    94
    90
    12 500
    2.5
    20
    [28-29]
    CaYAlO4 11 61 1 059
    1 045
    33
    156
    36
    740
    2.9
    19.2
    [30-31]
    Y3Al5O12 4 9 1 060
    1 051
    35
    100
    107
    151
    2.3
    3.2
    [32-33]
    SrY4(SiO4)3O 7 73 1 066
    1 068
    70
    94
    156
    110
    3.9
    3.1
    [34-35]
    Y2SiO5 6 48 1 041
    1 044
    122
    198
    410
    2 610
    2.7
    17.4
    [36]
    Lu2SiO5 6 67 1 059 233
    260
    1 100
    2 600
    7.3
    17.4
    [36]
    Gd2SiO5 6 72 1 031 343 396 7.9 [37]
    CaF2 18 71 1 049 65
    68
    35
    2 400
    3.2
    33
    [38-39]
    Na:CaF2 24/5 65/15 1 039 175
    190
    352
    510
    7.8
    6.6
    [40]
    YYF4 11 40 1 033
    1 031
    170
    210
    130
    250
    8.3
    14.3
    [41]
    YLiF4 11 40 1 028
    1 024
    196
    233
    54
    120
    1.4
    2.5
    [42]
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  • 收稿日期:  2019-11-18
  • 修回日期:  2019-12-20
  • 刊出日期:  2019-12-26

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