脉冲驱动等离子体射流中活性粒子空间分布规律

Spatial distribution of active particles in pulsed driven plasma jet

  • 摘要: 为探究大气压脉冲驱动等离子体射流中活性粒子空间分布特性,采用同轴双环等离子体射流反应器,在外施脉冲激励驱动下,研究各活性粒子在不同电离段的特征峰相对强度沿轴向空间的变化规律。结果表明:在脉冲激励等离子体射流所有测量点位均能检测到NO、OH、N2\rmN_2^+、He等活性粒子特征峰,其中以OH、N2\rmN_2^+粒子所对应的发射光谱谱带及特征峰较为显著;在高压电极和接地电极之间的电场驱动电离段,活性粒子NO、OH、N2的特征峰相对强度在靠近高压电极和接地电极区域较高,而在两电极中间的区域相对强度较低,不同激发能级He、\rmN_2^+特征峰相对强度沿气流方向逐渐降低;在接地电极至反应器管口的半开放离子激发段,活性粒子NO、OH以及不同能级N2\rmN_2^+、He特征峰的相对强度轴向分布呈现出随着气流方向逐渐降低的趋势;在反应器管口至等离子体射流末端区域的开放离子激发段,活性粒子OH、NO与不同能级He特征峰的相对强度轴向分布随气体流动方向逐渐减弱,不同能级N2\rmN_2^+特征峰的相对强度呈现出先增后减的规律,为脉冲驱动等离子体射流能量传递过程与反应机理的深入研究提供支撑。

     

    Abstract: To investigate the spatial distribution characteristics of active particles in atmospheric pressure pulse driven plasma jet, a coaxial double ring plasma jet reactor was used. Under external pulsed power excitation, the relative intensity changes of characteristic peaks of each active particle in different ionization regions along the axial space were studied. The results show that active particle characteristic peaks such as NO, OH, N2, \rmN_2^+, He, can be detected at all measurement points of the pulse excited plasma jet, with the emission spectral bands and characteristic peaks corresponding to OH, N2, \rmN_2^+ particles being more significant; In the upstream ionization section between the high-voltage electrode and the grounding electrode, the relative intensities of characteristic peaks of active particles NO, OH and N2 are higher near the high-voltage electrode and grounding electrode, while lower in the middle of the upstream ionization section. The relative intensities of characteristic peaks of different levels of He and \rmN_2^+ gradually decrease along the airflow direction; In the midstream ionization section from the grounding electrode to the reactor nozzle, the axial distribution of relative intensities of active particles NO, OH and characteristic peaks of different energy levels N2, \rmN_2^+ and He shows a gradually decreasing trend with the direction of the airflow; In the downstream ionization section from the reactor nozzle to the end of the plasma jet, the axial distribution of the relative intensity of the characteristic peaks of active particles OH and NO gradually weakens with the direction of gas flow; The relative intensity of the characteristic peaks of different energy levels N2, \rmN_2^+ and He shows a pattern of first increasing and then decreasing, providing strong support for the in-depth study of the energy transfer process and reaction mechanism of pulse driven plasma jet.

     

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