温/热稠密等离子体中的原子过程

Microscopic atomic processes in warm and hot dense plasmas

  • 摘要: 稠密等离子体广泛存在于天体内部及惯性约束聚变等高能量密度等离子体中,过去十几年的研究表明,目前学界主流的广泛使用的稠密等离子体中微观原子过程和宏观物理特性的理论,比如电离能下降、电子离子碰撞以及辐射不透明度等理论,难以有效处理复杂的稠密等离子体环境效应。本文系统回顾了稠密等离子体中微观原子过程相关的理论进展与面对最新实验结果的理论困难,介绍了我们建立的考虑了微观电子空间分布与非理想效应的自洽有限温度离子球屏蔽模型,并以温/热稠密条件下的电离能下降等实验验证了模型的正确性。除了研究得比较多的等离子体屏蔽效应之外,我们提出了原子过程中连续电子瞬时空间局域化的概念,建立了考虑瞬时空间局域化基础上的原子碰撞理论,并应用于研究稠密等离子体中的光电离、电子碰撞电离与电子碰撞激发以及俄歇衰变过程。研究结果表明,在稠密等离子体环境中发生的原子过程,在仅考虑等离子体屏蔽效应时,通常微观过程的截面会降低,但是,如果进一步包括瞬时空间局域化效应,那么光电离、电子碰撞电离与电子碰撞激发等连续原子过程的截面以及俄歇衰变速率随着等离子体密度的增高而显著增加。这些发现对理解、解释Z-箍缩装置上测量的铁等离子体不透明度大于理论预测等相关实验提供了宝贵线索,可望推动温/热稠密等离子体中微观原子过程和宏观物理特性的深入研究,为等离子体状态诊断与物理建模提供更精确的参数。

     

    Abstract: Dense plasmas are ubiquitous in stellar interiors and high-energy-density physics (HEDP) environments, such as inertial confinement fusion. Research over the past decade has demonstrated that the currently prevalent mainstream theories concerning microscopic atomic processes and macroscopic physical properties in dense plasmas—such as those addressing ionization potential depression (IPD), electron-ion collisions, and radiative opacity—struggle to effectively account for complex plasma environmental effects. This paper systematically reviews the theoretical advances related to microscopic atomic processes in dense plasmas, as well as the theoretical challenges posed by recent experimental results. We introduce the self-consistent finite-temperature ion-sphere (SCFTIS) screening model developed by our group, which incorporates microscopic electron spatial distributions and nonideal effects, and validate the accuracy of this model against experimental measurements of IPD under warm/hot dense conditions. Beyond the extensively studied plasma screening effects, we propose the concept of transient spatial localization of continuum electrons (TSLCE) in atomic processes. Building upon this concept, we have established an atomic collision theory that accounts for TSLCE and plasma screening and applied it to investigate photoionization, electron-impact ionization and excitation, and Auger decay processes in dense plasmas. Our findings indicate that for atomic processes occurring in dense plasma environments, the cross-sections of these microscopic processes typically decrease when only plasma screening effects are considered. However, when the TSLCE is further incorporated, the cross-sections for continuum atomic processes—such as photoionization, electron-impact ionization, and excitation—as well as Auger decay rates, exhibit a pronounced increase with elevated plasma density. These findings provide valuable insights for understanding and interpreting relevant experimental anomalies, such as the iron plasma opacity measured at the Z-pinch facility being higher than theoretical predictions. This work is expected to advance the fundamental research of microscopic atomic processes and macroscopic physical properties in warm/hot dense plasmas, thereby supplying more precise parameters for plasma diagnostics and physical modeling.

     

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