强脉冲中子的地面感生放射性环境研究

Study of the Ground-Induced Radioactive Environment Caused by Intense Pulsed Neutrons

  • 摘要: 强脉冲中子在地面产生的感生放射性γ辐射场受到源位置、地面介质组分的影响,呈现不同的分布特点,进而对人员造成不同程度的辐射危害。为评估不同场景(包括源位置与地面介质组成)下的感生放射性γ辐射环境水平,支撑强脉冲辐射环境研究与相关人员防护策略制定,基于大气分层模型,通过基于蒙卡的地面感生放射性两步计算方法计算了不同土壤条件下,感生放射性的剂量分布及典型位置剂量率随时间的变化规律,拟合给出了不同核素剂量贡献公式。通过对三种典型土壤的模拟计算,给出了核素活化系数以快速评估土壤中原子活化数,并通过单位质量剂量贡献评估了土壤中各种核素的平均剂量贡献;提出了土壤的安全驻留指数与安全驻留距离两个指标以在不同时间尺度下评价不同土壤条件下的强脉冲中子感生放射性环境的安全性。结果表明,源高度1000 m以下,剂量随源高度呈指数变化规律,且活化系数随水平投影距变化明显;单位质量Mn元素具有最高的剂量贡献,低Al土壤的土壤安全驻留指数更高,且Mn、Na元素含量高的土壤安全驻留距离更短。基于以上结果,计算了用于评价感生放射性在不同时间尺度对人员的安全影响的土壤安全指数与安全驻留距离参数,为后续差异化的安全策略提供数据支持。

     

    Abstract:
    Background The spatial distribution of the neutron-induced gamma radiation field generated within the ground medium by intense pulsed neutrons is critically dependent on the neutron source location and the chemical composition of the soil. These distributional variations give rise to differential radiological hazards for personnel.
    Purpose The objective of this study is to quantitatively assess the environmental levels of neutron-induced gamma radiation across diverse scenarios—specifically incorporating variations in neutron source location and ground medium composition—to facilitate research on intense pulsed neutron radiation environments and to inform evidence-based development of radiation protection protocols for personnel.
    Methods Based on an atmospheric stratification model, a two-step Monte Carlo simulation methodology was implemented to quantify the dose distribution of neutron-induced radioactivity within the ground medium and the temporal evolution of dose rates at representative locations across diverse soil compositions. Subsequently, empirical formulas characterizing the dose contributions of individual radionuclides were derived through curve-fitting analysis. Numerical simulations were performed for three representative soil compositions to derive nuclide-specific activation coefficients, facilitating rapid estimation of activated atom populations within the soil matrix. The average dose contributions of individual radionuclides were quantitatively evaluated based on dose contribution per unit mass. Furthermore, two novel safety metrics—the Soil Safety Residence Index and Safety Residence Distance —were proposed to systematically assess the safety of the induced radioactivity environment caused by intense pulsed neutron under varying soil conditions across multiple temporal scales.
    Results Results demonstrate that, for neutron source heights below 1000 m, the dose exhibits an exponential dependence on source altitude, while the activation coefficient shows pronounced variation with horizontal projection distance. Manganese (Mn) was identified as the element contributing the highest dose per unit mass. Soils with low aluminum (Al) content yielded a higher Soil Safety Residence Index, whereas soils enriched in manganese (Mn) and sodium (Na) exhibited shorter Safety Residence Distances, indicating elevated radiological risk under equivalent exposure conditions.
    Conclusions This study confirms that the spatial distribution and temporal evolution of the gamma radiation field generated by intense pulsed neutrons are governed by source geometry and the chemical composition of the soil medium. Manganese (Mn) is identified as the predominant radionuclide contributing to dose per unit mass, underscoring the imperative for enhanced radiological protection protocols in manganese-enriched soil environments. Moreover, the Soil Safety Residence Index and Residence Distance serve as rapid, quantitative metrics to inform appropriate radiation protection strategies for personnel across diverse soil conditions.

     

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